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Updated trends of the stratospheric ozone vertical distribution in the 60°S-60°N latitude range based on the LOTUS regression model

Sophie Godin-Beekmann 1, * Niramson Azouz 1 Viktoria Sofieva 2 Daan Hubert 3 Irina Petropavlovskikh 4 Peter Effertz 4 Gérard Ancellet 5 Doug Degenstein 6 Daniel Zawada 6 Lucien Froidevaux 7 Stacey Frith 8, 9 Jeannette Wild 10, 11 Sean Davis 12 Wolfgang Steinbrecht 13 Thierry Leblanc 7 Richard Querel 14 Kleareti Tourpali 15 Robert Damadeo 16 Eliane Maillard-Barras 17 René Stübi 17 Corinne Vigouroux 3 Carlo Arosio 18 Gerald Nedoluha 19 Ian Boyd 20 Roeland van Malderen 21 
Abstract : This study presents an updated evaluation of stratospheric ozone profile trends in the 60° S–60° N latitude range over the 2000–2020 period, using an updated version of the Long-term Ozone Trends and Uncertainties in the Stratosphere (LOTUS) regression model that was used to evaluate such trends up to 2016 for the last WMO Ozone Assessment (2018). In addition to the derivation of detailed trends as a function of latitude and vertical coordinates, the regressions are performed with the data sets averaged over broad latitude bands, i.e. 60° S–35° S, 20° S–20° N and 35° N–60° N. The same methodology as in the last Assessment is applied to combine trends in these broad latitude bands in order to compare the results with the previous studies. Longitudinally resolved merged satellite records are also considered in order to provide a better comparison with trends retrieved from ground-based records, e.g. lidar, ozone sondes, Umkehr, microwave and Fourier Transform Infrared (FTIR) spectrometers at selected stations where long-term time series are available. The study includes a comparison with trends derived from the latest REF-C2 simulations of the Chemistry Climate Model Initiative (CCMI). This work confirms past results showing an ozone increase in the upper stratosphere, which is now significant in the three broad latitude bands. The increase is largest in the northern and southern hemisphere midlatitudes, with ~2.2 %/decade at ~2.1 hPa, and ~2.1 %/decade at ~3.2 hPa respectively, compared to ~1.6 %/decade at ~2.6 hPa in the tropics. New trend signals have emerged from the records, such as a significant decrease of ozone in the tropics around 35 hPa and a non-significant increase of ozone in the southern mid-latitudes at about 20 hPa. Non-significant negative ozone trends are derived in the lowermost stratosphere, with the most pronounced trends in the tropics. While a very good agreement is obtained between trends from merged satellite records and the CCMI REF-C2 simulation in the upper stratosphere, observed negative trends in the lower stratosphere are not reproduced by models at southern and, in particular, at northern midlatitudes, where models report an ozone increase. However, the lower stratospheric trend uncertainties are quite large, for both measured and modelled trends. Finally, 2000–2020 stratospheric ozone trends derived from the ground-based and longitudinally resolved satellite records are in close agreement, especially over the European Alpine and tropical regions.
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Submitted on : Monday, March 14, 2022 - 6:43:22 PM
Last modification on : Friday, March 18, 2022 - 5:30:09 PM
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Sophie Godin-Beekmann, Niramson Azouz, Viktoria Sofieva, Daan Hubert, Irina Petropavlovskikh, et al.. Updated trends of the stratospheric ozone vertical distribution in the 60°S-60°N latitude range based on the LOTUS regression model. Atmospheric Chemistry and Physics Discussions, European Geosciences Union, 2022, pp.(Under Review). ⟨10.5194/acp-2022-137⟩. ⟨insu-03608514⟩



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