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Convective hydration in the tropical tropopause layer during the StratoClim aircraft campaign: pathway of an observed hydration patch

Abstract : The source and pathway of the hydration patch in the TTL (tropical tropopause layer) that was measured during the Stratospheric and upper tropospheric processes for better climate predictions (StratoClim) field campaign during the Asian summer monsoon in 2017 and its connection to convective overshoots are investigated. During flight no. 7, two remarkable layers are measured in the TTL, namely (1) the moist layer (ML) with a water vapour content of 4.8-5.7 ppmv in altitudes of 18-19 km in the lower stratosphere and (2) the ice layer (IL) with ice content up to 1.9 eq. ppmv (equivalent parts per million by volume) in altitudes of 17-18 km in the upper troposphere at around 06:30 UTC on 8 August to the south of Kathmandu (Nepal). A Meso-NH convection-permitting simulation succeeds in reproducing the characteristics of the ML and IL. Through analysis, we show that the ML and IL are generated by convective overshoots that occurred over the Sichuan Basin about 1.5 d before. Overshooting clouds develop at altitudes up to 19 km, hydrating the lower stratosphere of up to 20 km with 6401 t of water vapour by a strong-to-moderate mixing of the up-draughts with the stratospheric air. A few hours after the initial overshooting phase, a hydration patch is generated, and a large amount of water vapour (above 18 ppmv) remains at even higher altitudes up to 20.5 km while the anvil cloud top descends to 18.5 km. At the same time, a great part of the hydrometeors falls shortly, and the water vapour concentration in the ML and IL decreases due to turbulent diffusion by mixing with the tropospheric air, ice nucleation, and water vapour deposition. As the hydration patch continues to travel toward the south of Kathmandu, tropospheric tracer concentration increases up to ∼ 30 % and 70 % in the ML and IL, respectively. The air mass in the layers becomes gradually diffused, and it has less and less water vapour and ice content by mixing with the dry tropospheric air.
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Keun-Ok Lee, Thibaut Dauhut, Jean-Pierre Chaboureau, Sergey Khaykin, Martina Krämer, et al.. Convective hydration in the tropical tropopause layer during the StratoClim aircraft campaign: pathway of an observed hydration patch. Atmospheric Chemistry and Physics, European Geosciences Union, 2019, 19 (18), pp.11803-11820. ⟨10.5194/acp-19-11803-2019⟩. ⟨insu-02295170⟩

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