Estimates of ozone return dates from Chemistry-Climate Model Initiative simulations

Sandip Dhomse 1 Douglas Kinnison 2 Martyn Chipperfield 3 Ross Salawitch 4, 5, 6 Irene Cionni 7 Michaela Hegglin 8 N. Abraham 9, 10 Hideharu Akiyoshi 11 Alex Archibald 10, 9 Ewa Bednarz 9 Slimane Bekki 12 Peter Braesicke 13 Neal Butchart 14 Martin Dameris 15 Makoto Deushi 16 Stacey Frith 17, 18 Steven Hardiman 14 Birgit Hassler 15 Larry Horowitz 19 Rong-Ming Hu 12 Patrick Jöckel 15 Beatrice Josse 20 Oliver Kirner 21 Stefanie Kremser 22 Ulrike Langematz 23 Jared Lewis 22 Marion Marchand 12 Meiyun Lin 19, 24 Eva Mancini 25 Virginie Marecal 20 Martine Michou 20 Olaf Morgenstern 26 Fiona O'Connor 14 Luke Oman 18 Giovanni Pitari 27 David Plummer 28 John Pyle 9 Laura Revell 29 Eugene Rozanov 30, 29 Robyn Schofield 31 Andrea Stenke 29 Kane Stone 31 Kengo Sudo 32 Simone Tilmes 33 Daniele Visioni 34 Yousuke Yamashita 11 Guang Zeng 26
LATMOS - Laboratoire Atmosphères, Milieux, Observations Spatiales
24 AOS Program - Atmospheric and Oceanic Sciences Program [Princeton]
GFDL - NOAA Geophysical Fluid Dynamics Laboratory, Princeton University
Abstract : We analyse simulations performed for the Chemistry-Climate Model Initiative (CCMI) to estimate the return dates of the stratospheric ozone layer from depletion caused by anthropogenic stratospheric chlorine and bromine. We consider a total of 155 simulations from 20 models, including a range of sensitivity studies which examine the impact of climate change on ozone recovery. For the control simulations (unconstrained by nudging towards analysed meteorology) there is a large spread (±20 DU in the global average) in the predictions of the absolute ozone column. Therefore, the model results need to be adjusted for biases against historical data. Also, the interannual variability in the model results need to be smoothed in order to provide a reasonably narrow estimate of the range of ozone return dates. Consistent with previous studies, but here for a Representative Concentration Pathway (RCP) of 6.0, these new CCMI simulations project that global total column ozone will return to 1980 values in 2049 (with a 1σ uncertainty of 2043–2055). At Southern Hemisphere mid-latitudes column ozone is projected to return to 1980 values in 2045 (2039–2050), and at Northern Hemisphere mid-latitudes in 2032 (2020–2044). In the polar regions, the return dates are 2060 (2055–2066) in the Antarctic in October and 2034 (2025–2043) in the Arctic in March. The earlier return dates in the Northern Hemisphere reflect the larger sensitivity to dynamical changes. Our estimates of return dates are later than those presented in the 2014 Ozone Assessment by approximately 5–17 years, depending on the region, with the previous best estimates often falling outside of our uncertainty range. In the tropics only around half the models predict a return of ozone to 1980 values, around 2040, while the other half do not reach the 1980 value. All models show a negative trend in tropical total column ozone towards the end of the 21st century. The CCMI models generally agree in their simulation of the time evolution of stratospheric chlorine and bromine, which are the main drivers of ozone loss and recovery. However, there are a few outliers which show that the multi-model mean results for ozone recovery are not as tightly constrained as possible. Throughout the stratosphere the spread of ozone return dates to 1980 values between models tends to correlate with the spread of the return of inorganic chlorine to 1980 values. In the upper stratosphere, greenhouse gas-induced cooling speeds up the return by about 10–20 years. In the lower stratosphere, and for the column, there is a more direct link in the timing of the return dates of ozone and chlorine, especially for the large Antarctic depletion. Comparisons of total column ozone between the models is affected by different predictions of the evolution of tropospheric ozone within the same scenario, presumably due to differing treatment of tropospheric chemistry. Therefore, for many scenarios, clear conclusions can only be drawn for stratospheric ozone columns rather than the total column. As noted by previous studies, the timing of ozone recovery is affected by the evolution of N2O and CH4. However, quantifying the effect in the simulations analysed here is limited by the few realisations available for these experiments compared to internal model variability. The large increase in N2O given in RCP 6.0 extends the ozone return globally by ∼ 15 years relative to N2O fixed at 1960 abundances, mainly because it allows tropical column ozone to be depleted. The effect in extratropical latitudes is much smaller. The large increase in CH4 given in the RCP 8.5 scenario compared to RCP 6.0 also lengthens ozone return by ∼ 15 years, again mainly through its impact in the tropics. Overall, our estimates of ozone return dates are uncertain due to both uncertainties in future scenarios, in particular those of greenhouse gases, and uncertainties in models. The scenario uncertainty is small in the short term but increases with time, and becomes large by the end of the century. There are still some model–model differences related to well-known processes which affect ozone recovery. Efforts need to continue to ensure that models used for assessment purposes accurately represent stratospheric chemistry and the prescribed scenarios of ozone-depleting substances, and only those models are used to calculate return dates. For future assessments of single forcing or combined effects of CO2, CH4, and N2O on the stratospheric column ozone return dates, this work suggests that it is more important to have multi-member (at least three) ensembles for each scenario from every established participating model, rather than a large number of individual models.
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Submitted on : Friday, June 15, 2018 - 4:36:04 PM
Last modification on : Monday, January 13, 2020 - 4:30:03 PM

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Sandip Dhomse, Douglas Kinnison, Martyn Chipperfield, Ross Salawitch, Irene Cionni, et al.. Estimates of ozone return dates from Chemistry-Climate Model Initiative simulations. Atmospheric Chemistry and Physics, European Geosciences Union, 2018, 18 (11), pp.8409 - 8438. ⟨10.5194/acp-18-8409-2018⟩. ⟨insu-01816825⟩



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