Strategies for joint inversion of apatite fission track and (U-Th) data: application of radiation damage and fragment models.
Abstract
Apatite fission track (AFT) and (U-Th-Sm)/He (AHe)
thermochronology has the potential to constrain rock cooling
paths through a temperature range of c. 120 – 30°C. The annealing
behaviour of fission tracks in apatite has been well calibrated and
it has been shown that the annealing rate of tracks decreases with
temperature through a temperature range of 110 – 60°C. Retention
of He within apatite, however, occurs over a wide range of
temperatures with the closure temperature of an individual grain
being dependant on the grain size and, significantly, the amount of
radiation damage accumulated within the crystal.
The influence of radiation damage is particularly important for
apatite crystals that are enriched in U and Th and have
experienced protracted cooling histories over 10 – 100 million
year timescales. At present, current models of radiation damage
accumulation and annealing are not ideally parameterised for
natural apatites with high eU concentrations or complex
compositions. For this reason, single-grain AHe ages from high
eU and/or slowly cooled samples are typically highly dispersed
and poorly reproduced during thermal history inversion
modelling.
Here, we present new AHe data from samples collected from
Fennoscandia, which have resided at temperatures < 110ºC since
the Precambrian, and from South Africa, which have anomalously
high eU concentrations (e.g. up to 430 ppm). These data present
an opportunity to investigate the extreme cases of radiation
damage accumulation in natural samples. Using these data we
employ the latest radiation damage annealing model and vary key
parameters (e.g. trapping energy and Rmr0) to explore the
structural and compositional factors influencing helium diffusion
and explain the observed data. By integrating these AHe data with
independent AFT data and accounting for the different phenomena
causing single-grain age dispersion (e.g. radiation damage, grain
size, fragmentation) we can obtain robust thermal history
information from complex thermochronology data and better
understand single-grain age dispersion in geologically old settings