Worldwide spatiotemporal atmospheric ammonia (NH₃) columns variability revealed by satellite

Martin van Damme (1, 2) , Jan Willem Erisman (2, 3) , Lieven Clarisse (1) , Enrico Dammers (2) , Simon Whitburn (1) , Cathy Clerbaux (1, 4) , A. Johannes Dolman (2) , Pierre-François Coheur (1)

1 Spectroscopie de l'atmosphère, Service de Chimie Quantique et Photophysique
2 FALW - Faculty of Earth and Life Sciences [Amsterdam]
3 LBI - Louis Bolk Institute
4 TROPO - LATMOS

We exploit six years of measurements from the IASI/MetOp-A instrument to identify seasonal patterns and inter-annual variability of atmospheric NH₃. This is achieved by analyzing the time evolution of the monthly-mean NH₃ columns in 12 subcontinental areas around the world, simultaneously considering measurements from IASI morning and evening overpasses. For most regions, IASI has a sufficient sensitivity throughout the years to capture the seasonal patterns of NH₃ columns, and we show that each region is characterized by a well-marked and distinctive cycle, with maxima mainly related to underlying emission processes. The largest column abundances and seasonal amplitudes throughout the years are found in Southwestern Asia,with maxima twice as large as what is observed in Southeastern China. The relation between emission sources and retrieved NH₃ columns is emphasized at smaller regional scale by inferring a climatology of the month of maximum columns.

Mots clés: NH₃ source processes; seasonality; spatiotemporal variability; NH₃; N cycle; IASI satellite; ammonia

Domaines: Physique Atmosphérique et Océanique [physics.ao-ph]

Martin van Damme, Jan Willem Erisman, Lieven Clarisse, Enrico Dammers, Simon Whitburn, et al.. Worldwide spatiotemporal atmospheric ammonia (NH₃) columns variability revealed by satellite. Geophysical Research Letters, 2015, 42 (20), pp.8660-8668. ⟨10.1002/2015GL065496⟩. ⟨insu-01202973⟩